Quantum theory and relativity have shown the solid path for solid-state computation in the early 20th century. Since then, many theoretical breakthroughs accompanied by experimental discoveries have ultimately led us to this modern-day electronic society.

In this thesis, we focus on the design and development of 4D printed sensors. Carbon nanotubes (CNTs) are used as the active sensing medium as they have proven to be ideal for application in sensors due to their high electric conductivity, stability, and mechanical flexibility. The effect of a heat-shrinkable substrate on the electronic and structural properties of CNTs is analyzed in depth, followed by the application in temperature, humidity, and pressure sensors. The results show that the 4D effect results in a more porous yet more conductive film due to an increase in the charge carrier concentration, enabling an improved sensitivity of the devices and allowing us to tune the selectivity based on the shrinking percentage. The developed device was fabricated using a rapid, cost-effective technique that is independent of advanced fabrication facilities to expand its applications to low-resource settings and environments.